Log into GMail on a computer and see if there is some very large attachment that your phone is trying to download.
Other options might be to see if there is a message that has a lot of non-standard characters (extended ASCII characters, for example) or that is in a different language.
If you find any of those, move that particular email to a different folder that you do not have set up to sync, and then try synchronizing again on your phone.
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